Whaetley from Portal 2!! One of the biggest emotional rides of my life

Also Jillius, but he wasn't
really the villain so

and I'm not sure how I feel about Janga... He's awesome but at the same time he orphaned a wolf pup ;-;
And I musn't forget Ales Mansay!! He's probably one of my favorite villains (and Rayman characters) of all time!!